This is an easy way to catch Mesprit. It only works after having encountered Palkia/Dialga and defeating Team Galactic. Mesprit is located in Lake Verity. After going into the cave to find him, you will encounter Mesprit and he will fly away. Then the Professor will come up to you and tell you that Mesprit wants to play chase with you. After that, you should...
Go to Jubilife City and get the map marker app in the Poketech building.
There will be a marker on the map that looks like Mesprit.
Do whatever until the marker is on one of the routes next to you.
Chase him down and look in grass to start the battle if his marker is on top of yours.
Once in battle, use a fast Pokémon to use Mean Look or throw a Master Ball.
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